塔克拉玛干沙漠腹地黑碳气溶胶浓度

doi:10.7522/j.issn.1000-694X.2013.00409

摘要/Abstract

摘要： 利用2006年3月-2007年2月塔克拉玛干沙漠腹地塔中气象站黑碳测量仪的观测数据，结合同期PM₁₀、能见度及常规气象观测资料，分析了沙漠地区大气中黑碳气溶胶浓度的变化特征及其影响因子。结果表明：观测期间黑碳浓度小时平均值为1.81±1.58 μg·m^-3，日平均浓度为1.72±0.85 μg·m^-3，区域本底值为0.78 μg·m^-3；日变化呈单峰，与其他地区的双峰、三峰型不同；季节变化特征明显，春、冬季黑碳浓度较高，秋季较低，春季大量沙尘增加了气溶胶的吸收特性，黑碳测量仪观测的黑碳浓度要高于近地面大气中实际的黑碳浓度；黑碳浓度小时平均值与风速呈显著非线性相关，不同风向下黑碳浓度水平有较明显的差异，该地区黑碳浓度的变化与盛行风向上来自污染较严重地区的气团输送有关，并且受局地沙尘和排放源的影响。

关键词: 黑碳气溶胶, 黑碳测量仪, 观测, 影响因子

Abstract: The black carbon aerosol mass concentrations were continuously observed by aethalometer at Tazhong meteorological station in the hinterland of the Taklimakan Desert from March of 2006 to February of 2007, and in combining with the data of mass concentrations of PM₁₀, visibility and the routine weather observation, the variation features of black carbon and influencing factors were analyzed in this paper. The results showed that the hourly and daily average values of black carbon concentration were 1.81±1.58 g·m^-3and 1.72±0.85 g·m^-3, separately, and the regional background concentration of black carbon was 0.78 g·m^-3; the diurnal variation of black carbon mass concentration showed a single peak curve, which is different from the double or three peak curve in other areas; the seasonal variation of black carbon concentration was obvious, which was higher in spring and winter, lower in autumn; due to the aerosol absorption increased by heavy dust in spring, the black carbon mass concentrations observed by Aethalometer would be higher than actual values of the near surface; the hourly average black carbon concentrations were significantly non-linearly correlated with wind speed and the black carbon concentrations obviously differed in various wind directions; the local variation of the black carbon concentrations were relevant to the seriously polluted air mass transported from the prevailing wind direction, and were affected by the local dust and emission sources.

Key words: black carbon aerosol, aethalometer, observation, influencing factor

中图分类号:

O648.18

陆辉, 魏文寿, 崔彩霞, 吴新萍. 塔克拉玛干沙漠腹地黑碳气溶胶浓度[J]. 中国沙漠, 2014, 34(4): 1087-1093.

Lu Hui, Wei Wenshou, Cui Caixia, Wu Xinping. Concentration of Black Carbon in the Hinterland of the Taklimakan Desert[J]. JOURNAL OF DESERT RESEARCH, 2014, 34(4): 1087-1093.

参考文献

[1] Berner A,Sidla S,Galambos Z,et al.Modal character of atmospheric black carbon size distributions[J].Journal of Geophysical Research,1996,101(D14):19559-19565.
[2] Wolff G T.Particulate elemental carbon in the atmosphere[J].Journal of the Air Pollution Control Association,1981,31(9):935-938.
[3] Goldberg E D.Black Carbon in the Environment:Properties and Distribution[M].New York,USA:John Wiley,1985:2.
[4] Cooke W F,Wilson J N.A global black carbon aerosol model[J].Journal of Geophysical Research,1996,101(D14):19395-19409.
[5] IPCC.Climate Change 2007:The Physical Science Basis[R].Cambridge,UK:Cambridge University Press,2007:163-167.
[6] Qiu J,Yang L.Variation characteristics of atmospheric aerosol optical depths and visibility in North China during 1980-1994[J].Atmospheric Environment,2000,34(4):603-609.
[7] Park R J,Jacob D J,Chin M,et al.Sources of carbonaceous aerosols over the United States and implications for natural visibility[J].Journal of Geophysical Research,2003,108(DI2):4355.
[8] Hansen A D A.The Aethalometer Manual[Z].Berkeley,USA:Magee Scientific,2003:21.
[9] Alfaro S C,Gomes L,Rajot J L,et al.Chemical and optical characterization of aerosols measured in spring 2002 at the ACE-Asia supersite,Zhenbeitai,China[J].Journal of Geophysical Research,2003,108(D23):8641.
[10] Lelieveld J,Crutzen P J,Ramanathan V,et al.The Indian Ocean experiment:widespread air pollution from south and southeast Asia[J].Science,2001,291(5506):1031-1036.
[11] Kleefeld S,Hoffer A,Z Krivácsy,et al.Importance of organic and black carbon in atmospheric aerosols at Mace Head,on the West Coast of Ireland (53°19'N,9°54'W)[J].Atmospheric Environment,2002,36(28):4479-4490.
[12] Hansen A D A,Lowenthal D H,Chow J C,et al.Black carbon aerosol at McMurdo station,Antarctica[J].Journal of the Air & Waste Management Association,2001,51(4):593-600.
[13] Lavanchy V M H,Gäggeler H W,Nyeki S,et al.Elemental carbon (EC) and black carbon (BC) measurements with a thermal method and an aethalometer at the high-alpine research station Jungfraujoch[J].Atmospheric Environment,1999,33(17):2759-2769.
[14] Shah J J,Johnson R L,Heyerdahl E K,et al.Carbonaceous aerosol at urban and rural sites in the United States[J].Journal of the Air Pollution Control Association,1986,36(3):254-257.
[15] 汤洁,温玉璞,周凌晞,等.中国西部大气清洁地区黑碳气溶胶的观测研究[J].应用气象学报,1999,10(2):160-170.
[16] 杨东贞,于晓岚,李兴,等.临安大气污染本底站气溶胶特征分析[J].大气科学,1995,19(2):119-227.
[17] 秦世广.我国大陆地区大气黑碳气溶胶观测研究[D].北京:中国气象科学研究院,2001.
[18] 柯宗建.我国东部地区气溶胶光学特征观测研究[D].北京:中国气象科学研究院,2004.
[19] 娄淑娟,毛节泰,王美华.北京地区不同尺度气溶胶中黑碳含量的观测研究[J].环境科学学报,25(1):17-22.
[20] 杨溯,张武,韩晶晶,等.上海市浦东新区秋冬季黑碳气溶胶特性[J].兰州大学学报(自然科学版),2008,44(4):66-70.
[21] 李杨,曹军骥,张小曳,等.2003年秋季西安大气中黑碳气溶胶的演化特征及其来源解析[J].气候与环境研究,2005,10(2):230-237.
[22] 陶俊,朱李华,韩静磊,等.2007年春季广州城区黑碳气溶胶污染特征的初步研究[J].气候与环境研究,2008,13(5):658-662.
[23] 吴兑,毛节泰,邓雪娇,等.珠江三角洲黑碳气溶胶及其辐射特性的观测研究[J].中国科学 D辑:地球科学,2009,52(8):1152-1163.
[24] 章秋英,牛生杰,沈建国,等.半干旱区冬春季黑碳气溶胶吸收特性的观测研究[J].中国沙漠,2009,29(1):183-188.
[25] 杨溯,张武,史晋森,等.半干旱地区黑碳气溶胶特征初步分析[J].气候与环境研究,2010,15(6):756-764.
[26] 王旭,马禹,陈洪武,等.南疆沙尘暴气候特征分析[J].中国沙漠,2003,23(2):147-151.
[27] Gao Y,Arimoto R,Duce R A,et al.Temporal and spatial distribution of dust and its deposition to the China Sea[J].Tellus B,1997,49(2):172-189.
[28] Pakkanen T A,Kerminen V M,Ojanen C H,et al.Atmospheric black carbon in Helsinki[J].Atmospheric Environment,2000,34:1497-1506.
[29] Bhugwant C,Cachier H,Bessafi M,et al.Impact of traffic on black carbon aerosol concentration at La Réunion Island (Southern Indian ocean)[J].Atmospheric Environment,2000,34(20):3463-3473.
[30] 缪启龙,王晶,何清,等.南疆沙漠腹地大气边界层气象要素廓线分析[J].气象与减灾研究.2009,32(2):6-10.
[31] 李祥余,何清,黄少鹏,等.南疆一次强沙尘暴前后塔中近地面各气象要素的变化特征[J].高原气象,2009,28(3):652-662.
[32] 刘新春,钟玉婷,何清,等.塔克拉玛干沙漠腹地沙尘气溶胶质量浓度垂直分布特征[J].中国沙漠,2012,32(4):1045-1052.
[33] 刘新春,钟玉婷,何清,等.塔克拉玛干沙漠腹地及周边地区PM-10时空变化特征及影响因素分析[J].中国沙漠,2011,31(2):323-330.
[34] 高润祥,牛生杰,张华,等.2006年春季西北地区黑碳气溶胶的观测研究[J].南京气象学院学报,2008,31(5):655-661.
[35] Fialho P,Hansen A D A,Honrath R E.Absorption coefficients by aerosols in remote areas:a new approach to decouple dust and black carbon absorption coefficients using seven wavelength aethalometer data[J].Joumal of Aerosol Science,2005,36:267-282.
[36] Lu H,Wei W S,Liu M Z,et al.Aerosol optical absorption by dust and black carbon in Taklimakan Desert,during no-dust and dust-storm conditions[J].Particuology,2012,10(4):509-516.
[37] Hansen A D A,Bodhaine B A,Dutton E G,et al.Aerosol black carbon measurements at the South Pole:initial results 1986-1987[J].Geophysical Research Letters,1988,15(11):1193-1196.
[38] Ogren J A,Groblicki P J,Charlson R J.Measurement of the removal rate of elemental carbon from the atmosphere[J].Science of the Total Environment,1984,36:329-338.
[39] Bahrmann C P,Saxena V K.Influence of air mass history on black carbon concentration in the southeastern United States[J].Journal of Geophysical Research,1998,103(D18):23153-23161.
[40] Liousse C,Penner J E,Chuang C,et al.A global three-dimensional model study of carbonaceous aerosols[J].Journal of Geophysical Research.1996,101(D14):19411-19432.
[41] Babu S S,Moorthy K K.Anthropogenic impact on aerosol black carbon mass concentration at a tropical coastal station:a case study [J].Current Science,2001,81(9):1208-1214.
[42] 汤洁,颜鹏,秦世广,等.中国地区黑碳气溶胶的观测和研究[C]//第十二届全国大气环境学术会议论文集.辽宁丹东,2005:296-304.
[43] Järvi L,Junninen H,Karppinen A,et al.Temporal variations in black carbon concentrations with different time scales in Helsinki during 1996-2005[J].Atmospheric Chemistry Physics,2008,8:10l7-1027.
[44] 李江风.塔克拉玛干沙漠和周边山区天气气候[M].北京:科学出版社,2003:190.
[45] 薛福民,刘新春,马燕,等.1997-2007年塔克拉玛干沙漠腹地沙尘天气变化特征[J].沙漠与绿洲气象,2009,3(1):31-34.
[46] 陆辉,魏文寿,崔彩霞.塔克拉玛干沙漠腹地黑碳气溶胶与气象因子及其来源的初步研究[C]//第29届中国气象学会年会“大气成分与天气气候变化”分会场论文集.辽宁沈阳,2012.
[47] 薛福民,李娟,黄侃,等.塔克拉玛干沙漠黑碳气溶胶的特性及来源[J].中国科学:化学,2010,40(5):556-566.