img

官方微信

  • CN 62-1070/P
  • ISSN 1000-694X
  • 双月刊 创刊于1981年
高级检索
天气与气候

北京市大兴区大气降尘环境磁学特征及其环境意义

  • 田世丽1 ,
  • 夏敦胜1 ,
  • 2 ,
  • 余 晔1 ,
  • 王 博2 ,
  • 许淑婧2
展开
  • 1.中国科学院寒区旱区环境科学与工程研究所, 甘肃 兰州 730000;
    2.兰州大学 西部环境教育部重点实验室, 甘肃 兰州 730000

收稿日期: 2012-03-30

  修回日期: 2012-05-23

  网络出版日期: 2012-05-23

Magnetic Characteristics of Dustfall in Daxing District, Beijing, China and Its Environmental Implications

  • TIAN Shi-li1 ,
  • XIA Dun-sheng1 ,
  • 2 ,
  • YU Ye1 ,
  • WANG Bo2 ,
  • XU Shu-jing2
Expand
  • 1.Cold and Arid Regions Environmental and Engineering Research Institute, Chinese Academy of Sciences, Lanzhou 730000, China;
    2.Ministry of Education Key Laboratory of Western Chinas Environmental System, Lanzhou University, Lanzhou 730000, China

Received date: 2012-03-30

  Revised date: 2012-05-23

  Online published: 2012-05-23

摘要

应用环境磁学方法对北京市大兴区大气降尘环境磁学特征进行了系统研究,并通过与北京市朝阳区、兰州市大气降尘环境磁学特征的对比,对环境磁学在污染物来源解析及扩散条件研究中的应用机理进行了探讨。结果表明,大兴区大气降尘磁性矿物含量明显高于本区表土,人为源影响显著;降尘样品磁学特征主要受磁铁矿控制,并含有一定数量的磁赤铁矿,磁性矿物为准单畴和多畴颗粒;大兴区降尘样品的磁性矿物含量明显低于朝阳区,且样品颗粒相对较细,表明人口密度、车流量、城市发达度对大气污染程度存在显著影响;大兴区与兰州市大气降尘磁性矿物含量的季节变化差异表明,燃煤取暖对北京大气质量的影响显著减弱,燃煤锅炉改造是大气污染防治的重要措施之一。气象因素对大气颗粒物浓度变化有重要影响,降水、低气压和高风速利于大气颗粒物的清除和扩散,低气温对大气颗粒物污染的负面影响显著。

本文引用格式

田世丽1 , 夏敦胜1 , 2 , 余 晔1 , 王 博2 , 许淑婧2 . 北京市大兴区大气降尘环境磁学特征及其环境意义[J]. 中国沙漠, 2013 , 33(3) : 832 -839 . DOI: 10.7522/j.issn.1000-694X.2013.00119

Abstract

We investigated the magnetic characteristics of the dustfall samples collected from Daxing District of Beijing by using the magnetic methods.Furthermore, we explored the application of environmental magnetism to the source apportionment and diffusion of pollutants based on the comparison of the magnetic analysis results to that of dustfall sampled from Chaoyang District of Beijing and Lanzhou, respectively.The results reveal that the concentration of magnetic mineral in dustfall sampled from Daxing District is much higher than that in the topsoil of the same area. The main magnetic minerals in the dustfall are magnetite and maghemite, and the main magnetic grain sizes are mainly pseudo single-domain(PSD) and multi-domain(MD). The content of magnetic mineral in dustfall sampled from Chaoyang District is much higher than that from Daxing District, which implies that air pollution was significantly affected by population density, traffic condition and the urbanization level. The seasonal variability of the content of magnetic mineral in dustfall sampled from Daxing District and Lanzhou  indicates that the air quality of Beijing has been improved by the reduced impacts of coal-firing. Inferred from meteorological data, we found that local precipitation, low pressure and high wind speed were conducive to the removal as well as diffusion of atmospheric particulate matter, while low temperature has a significant negative impact on that.

参考文献

[1]奚旦立,孙裕生,刘秀英.环境监测[M].第3版.北京:高等教育出版社,2002.

[2]贾晓鹏,石晓萌,王海兵.降尘过程指示的沙尘循环过程[J].中国沙漠,2012,32(3):600-603.

[3]赵伦.大气颗粒物对人体健康影响的研究进展[J].山东环境,1997,(1):44-45.

[4]刘新春,钟玉婷,何清,等.塔克拉玛干沙漠腹地沙尘暴过程大气颗粒物浓度及影响因素分析[J].中国沙漠,2011,31(6):1548-1553.

[5]Stone E,Schauer J,Quraishi T A,et al.Chemical characterization and source apportionment of fine and coarse particulate matter in Lahore,Pakistan[J].Atmospheric Environment,2010,44(8):1062-1070.

[6]Karanasiou A A,Siskos P A,Eleftheriadis K.Assessment of source apportionment by Positive Matrix Factorization analysis on fine and coarse urban aerosol size fractions[J].Atmospheric Environment,2009,43(21):3385-3395.

[7]Song F,Gao Y.Chemical characteristics of precipitation at metropolitan Newark in the US East Coast[J].Atmospheric Environment,2009,43(32):4903-4913.

[8]Sakihama H,Ishiki M,Tokuyama A.Chemical characteristics of precipitation in Okinawa Island,Japan[J].Atmospheric Environment,2008,42(10):2320-2335.

[9]Thompson R,Oldfield F.Environmental Magnetism[M].Lonton:Allen Unwin,1986.

[10]王博,夏敦胜,余晔,等.兰州市城区河道表层沉积物磁性特征研究[J].环境科学,2010,31(8):1740-1748.

[11]Zhao X Y,Liu Q S.Effects of the grain size distribution on the temperature-dependent magnetic susceptibility of magnetite nanoparticles[J].Science China:Earth Sciences,2010,(7):1071-1078.

[12]Wang H Q,Zhang S H,Li H Y.Mineral magnetic properties of surface sediments at Bei’anhe,Beijing,and its environmental significance[J].Chinese Science Bulletin,2008,(16):2536-2546.

[13]Wang G,Xia D S,Liu X M,et al.Spatial and temporal variation in magnetic properties of street dust in Lanzhou City,China[J].Chinese Science Bulletin,2008,(12):1913-1923.

[14]Gautam P,Blaha U,Appel E.Magnetic susceptibility of dust-loaded leaves as a proxy of traffic-related heavy metal pollution in Kathmandu city,Nepal[J].Atmospheric Environment,2005,39(12):2201-2211.

[15]Maher B A,Moore C,Matzka J.Spatial variation in vehicle-derived metal pollution identified by magnetic and elemental analysis of roadside tree leaves[J].Atmospheric Environment,2008,42(2):364-373.

[16]Muxworthy A R,Matzka J,Petersen N.Comparison of magnetic parameters of urban atmospheric particulate matter with pollution and meteorological data[J].Atmospheric Environment,2001,35(26):4379-4386.

[17]Xia D S,Chen F H,Bloemendal J,et al.Magnetic properties of urban dustfall in Lanzhou,China,and its environmental implications[J].Atmospheric Environment,2008,42(9):2198-2207.

[18]王丽,夏敦胜,余晔,等.北疆地区城市大气降尘磁学特征及其环境意义[J].中国沙漠,2010,30(3):699-705.

[19]Shu J,Dearing J A,Morse A P,et al.Determining the sources of atmospheric particles in Shanghai,China,from magnetic and geochemical properties[J].Atmospheric Environment,2001,35(15):2615-2625.

[20]杨丽萍,陈发虎.兰州市大气降尘污染物来源研究[J].环境科学学报,2002,(4):499-502.

[21]贾佳,夏敦胜,魏海涛,等.阿西克剖面记录的西天山地区黄土磁学性质及古气候意义初探[J].中国沙漠,2011,31(6):1406-1415.

[22]邓少福,杨太保,秦宏毅,等.新疆塔城黄土古土壤磁化率特征及其影响因素[J].中国沙漠,2011,31(4):848-854.

[23]Dearing J A,Bird P M,Dann R J L,et al.Secondary ferrimagnetic minerals in Welsh soils:a comparison of mineral magnetic detection methods and implications for mineral formation[J].Geophysical Journal International,1997,130:727-736.

[24]Day R,Fuller M,Schmidt V A.Hysteresis properties of titanomagnetites:Grain-size and compositional dependence[J].Physics of The Earth and Planetary Interiors,1977,13(4):260-267.

[25]Oldfield F,Yu L Z.The influence of particle size variations on the magnetic properties of sediments from the north-eastern Irish Sea[J].Sedimentology,1994,41:1093-1108.

[26]Peters C,Dekkers M J.Selected room temperature magnetic parameters as a function of mineralogy,concentration and grain size[J].Physics and Chemistry of the Earth,Parts A/B/C,2003,28(16/19):659-667.

[27]Peters C,Thompson R.Magnetic identification of selected natural iron oxides and sulphides[J].Journal of Magnetism and Magnetic Materials,1998,183(3):365-374.

[28]郑妍,张世红.北京市区尘土与表土的磁学性质及其环境意义[J].科学通报,2007,(20):2399-2406.

[29]乔庆庆,张春霞,李静,等.北京市朝阳区大气降尘磁学特征及对空气污染物浓度的指示[J].地球物理学报,2011,54(1):151-162.

[30]田世丽,夏敦胜,余晔,等.西北地区河谷城市大气降尘环境磁学特征及其环境意义[J].环境科学,2011,32(9):2761-2768.

[31]于令达,王广甫,朱光华,等.2008年北京采暖开始前后大气颗粒物化学成分及来源研究[J].环境科学学报,2010,30(1):204-210.

[32]章文波,陈红艳.实用数据统计分析及SPSS12.0应用[M].北京:人民邮电出版社,2006.

文章导航

/